介觀微粒庫倫液體之流變學

以作者查詢圖書館館藏

、以作者查詢臺灣博碩士

、以作者查詢全國書目

、勘誤回報

、線上人數：73

、訪客IP：3.147.60.62

姓名

詹佳玲(Chia-Ling Chan) 查詢紙本館藏

畢業系所

物理學系

論文名稱

介觀微粒庫倫液體之流變學
(Microrheology of Mesoscopic Dusty Coulomb Liquids)

相關論文

★ 二加一維鏈狀微粒電漿液體微觀運動與結構之實驗研究	★ 剪力下的庫倫流體微觀黏彈性反應
★ 強耦合微粒電漿中的結構與動力行為研究	★ 脈衝雷射誘發之雷漿塵爆
★ 強耦合微粒電漿中脈衝雷射引發電漿微泡	★ 二維強耦合微粒電漿方向序的時空尺度律
★ 二維微粒庫倫液體中集體激發微觀動力研究	★ 超薄二維庫侖液體的整齊行為
★ 超薄二維微粒電漿庫侖流的微觀運動行為	★ 微米狹縫中之脈衝雷射誘發二維氣泡相互作用
★ 二維神經網路系統之集體發火動力學行為	★ 大白鼠腦皮質層神經元網路之同步發放行為研究
★ 二維團簇腦神經網路之同步發火	★ 二維微粒電漿液體微觀結構之記憶行為
★ 微粒電漿中電漿微泡的生成與交互作用之動力行為研究	★ 脈衝雷射誘發雙氣泡間薄液層之不穩定性

檔案

[Endnote RIS 格式]

[Bibtex 格式]

[相關文章]

[文章引用]

[完整記錄]

[館藏目錄]

[檢視]

[下載]

本電子論文使用權限為同意立即開放。
已達開放權限電子全文僅授權使用者為學術研究之目的，進行個人非營利性質之檢索、閱讀、列印。
請遵守中華民國著作權法之相關規定，切勿任意重製、散佈、改作、轉貼、播送，以免觸法。

摘要(中)

摘要
在奈米科學中，介觀液體在狹縫中的微觀動力行為與其流變反應，
一直都是個很重要的議題。然而，由於測量尺度的限制，大多數的科學
家只能透過電腦模擬或者在實驗上，量測其表面力與速度等巨觀特性。
其微觀結構與運動行為，卻鮮少人能直接測量並探討研究。
在微粒庫倫系統中，我們將微粒丟入充滿電漿的二維長形空腔中。
由於電子有較高的遷移率，故空腔與微粒會帶負電，透過庫倫力的交互
作用，進而形成二維長形庫倫結構。藉由調控背景擾動，並輔以光學顯
微鏡，我們不僅能透過追蹤粒子的運動軌跡直接觀察到微粒庫倫液體的
狀態並且能觀測了解其微觀結構排列行為。
我們利用平行反向的雷射光束施加剪力在介觀庫倫液體的兩側，在
粒子間的相互影響，邊界效應，背景擾動，與外加剪力的交互作用，我
們發現其平均速度分布會分隔成兩區: 兩側高速度區夾著中間低速度
區。這種現象稱做”剪力帶的形成” 。透過一些統計工具的計算分
析(例如: 速度分布﹑結構變化率﹑以及一些時空關聯函數等等…)，我
們深入探討介觀液體形成剪力帶的起源並加以比較與其他系統(如: 玻
璃態的物質等...) 的異同特性。

摘要(英)

Abstract
We investigate experimentally the generic microscopic dynamical
behavior of a dust Coulomb liquid confined in a narrow mesoscopic
channel and sheared by two parallel counter laser beams along the
opposite boundaries, at the low stress limit where the shear induced
average speed is comparable to the thermal speed. A liquid confined in
a narrow channel with width down to the molecular scale usually exhibits
anomalous behavior in structure and motion deviating from the
bulk liquid, under the e®ect of discreteness, finite boundary, and lager
thermal fluctuations. It is an interesting and important issue for nanoscience
and technology. Nevertheless, the rheology studies have been
mainly limited to the macroscopic force and velocity measurement on
the confining boundary because of the lack of microscopic measures
at the small atomic scale, which is insu±cient to construct an obvious
microscopic picture for the sheared flow in a narrow channel. A dust
Coulomb liquid formed by micrometer sized dust particles charged
and suspended in a low pressure weakly ionized discharge background
is an heuristic system to mimic and understand the generic dynamical
behaviors at the kinetic level because of the capability of directly
visualization. In this work, through monitoring the spatio-temporal
evolution of micro-motion and correlating with the local structure rearrangement,
we demonstrate the following findings:
1. The mean velocity profile exhibits shear bands with high mean
shear rates in the outer region sandwiching a center zone with
low shear rate.
2. Stress enhanced avalanche type cooperative topological rearrangement
associated with the vortex type cooperative hopping involvi
ing a cluster of particles are observed in the shear band, which
are responsible for the observed enhanced longitudinal and transverse
velocity fluctuations and the higher structural relaxation
rate in the shear bands. It screens the external drive through
relaxing the local stress and leaves a weakly perturbed center
zone.
3. We also point out that the nonlinear threshold type stick-slip
hopping after accumulation of local stress is the origin for shear
thinning and shear banding which have also been observed in
glassy systems under the slow dynamics. Unlike in the glassy
system, the finite temperature e®ect leads to the absence of a
finite yield stress.

關鍵字(中)

★ 庫倫液體
★ 微粒

關鍵字(英)

★ Dusty Coulomb Liquids
★ Mesoscopic

論文目次

Contents
1 Introduction 1
2 Background and Theory 6
2.1 Rheology of Fluids . . . . . . . . . . . . . . . . . . . . . . . . 6
2.1.1 Rheology of Newtonian fluids . . . . . . . . . . . . . . 6
2.1.2 Rheology of non-Newtonian fluids . . . . . . . . . . . 7
2.1.3 Glassy rheology . . . . . . . . . . . . . . . . . . . . . . 8
2.2 Liquids in a Mesoscopic Channel . . . . . . . . . . . . . . . . 9
2.2.1 The microscopic picture of the bulk liquid . . . . . . . 9
2.2.2 Characteristics of a confined liquid . . . . . . . . . . . 10
2.3 Dusty Plasma System . . . . . . . . . . . . . . . . . . . . . . . 11
2.3.1 RF glow discharges and dusty plasma . . . . . . . . . . 11
2.3.2 The quasi-2D strongly coupled dusty plasma liquid . . 13
2.4 Topological Defects and Spatiotemporal Correlation Functions 15
2.4.1 Topological defects . . . . . . . . . . . . . . . . . . . . 15
2.4.2 Spatiotemporal correlation of local bond-orientational
order . . . . . . . . . . . . . . . . . . . . . . . . . . . 16
3 Experiment 21
3.1 Experimental Setup and Data Analysis . . . . . . . . . . . . . 21
iii
CONTENTS
4 Result and Discussion 26
4.1 Shear-free Coulomb Liquids . . . . . . . . . . . . . . . . . . . 26
4.1.1 The motion of microscopic liquids . . . . . . . . . . . . 27
4.1.2 Boundary e®ect for a confined liquid . . . . . . . . . . 27
4.2 Sheared Dusty Plasma Liquids . . . . . . . . . . . . . . . . . . 32
4.2.1 Nonlinear velocity response and the observation of shear
banding . . . . . . . . . . . . . . . . . . . . . . . . . . 32
4.2.2 Histogram of displacement . . . . . . . . . . . . . . . 36
4.3 The Generic Behavior of Shear Banding . . . . . . . . . . . . 37
4.3.1 Local structural rearrangement . . . . . . . . . . . . . 41
4.3.2 Temporal correlation of bond-orientation order . . . . . 42
4.3.3 The microscopic origin of shear banding . . . . . . . . 46
5 Conclusions 50

參考文獻

[1] e.g. S. Granick, Phys. Today, 52, No,7,26 (1999).
[2] e.g. J. Gollub, Phys, Today, 56, (1),10 (2003).
[3] C. L. Rhykerd, Jr., etal , Nature (London) 330, 461 (1987).
[4] P. A. Thompson, G. S. grest, and M. O. Robbins, Phys. Rev. Lett. 68,
3448 (1992).
[5] M. Heuberger, M. Zach, and N. d. Spencer, Science 292, 905 (2001).
[6] J. Gao, W. D. Luedtke, and U. Landman, Phys. Rev. Lett. 79, 705
(1997).
[7] A. L. Demirel and S. Granick, Phys. Rev. Lett. 77, 2261 (1996).
[8] L. W. Teng, P. S. Tu, and Phys. Rev. Lett. 90, 245004 (2003).
[9] e.g. T. E. Faber, FluuidDynamicsforPhysicsts (Cambridge University
Press, Cambridge, 1995).
[10] A. Kabla and G. Debregeas, Phys. Rev. Lett. 90, 258301 (2003).
[11] J. B. Salmon, A. C. Colin, and S. Manneville, Phys. Rev. Lett. 90,
228303 (2003).
53
Bibliography
[12] F. Varnik, L. Bocquet, J.-L. Barrat, and L. Berthier, Phys. Rev. Lett.
90, 095702 (2003).
[13] Y. Jiang, etal , Phys. Rev. E. 59, 5819 (1999).
[14] J. H. Chu and Lin I, Phys. Rev. Lett. 72, 4009 (1994).
[15] Y. J. Lai and Lin I, Phys. Rev. Lett. 89, 155002 (2002).
[16] K. J. Strandburg, Bond ¡ OrientationalOrderinCondensedMatterSystems
(Springer, New York, 1992).
[17] W. Y. Woon and Lin I, Phys. Rev. Lett. 92, 065003 (2004).
[18] Lin I, W. T. Juan, and C. H. Clnang, Science 272, 1626 (1996)
[19] P. Tapadia and S. Q. Wang, Phys. Rev. Lett. 91, 198301 (2003).
[20] G. Debregeas, H. Tabuteau and J.-M. di Meglio, Phys. Rev. Lett. 87,
178305 (2001).
[21] Y. J. Lai, Ph. D. thesis, National Central University, Republic of China,
(2002).

指導教授

伊林(Lin I)

審核日期

2004-7-5

推文