博碩士論文 105322044 詳細資訊




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姓名 林志鴻(Zhi-Hong Lin)  查詢紙本館藏   畢業系所 土木工程學系
論文名稱 深地層處置場緩衝材料小型熱-水-力耦合實驗精進與模擬比對
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摘要(中) 利用核能發電已經為世界各國主要電力來源之一,但是核子燃料具有高放射性,且半衰期長達數千年甚至數十萬年,而在衰變過程中產生之衰變熱,會對周圍產生溫度場效應,如何將用過核子燃料與生物圈完全隔絕,是各核能先進國家之共同目標。目前對於用過核子燃料處置方式一致較推崇「深地層處置」(Deep Geologic Disposal)概念,用以隔絕與減緩放射性核種釋放遷移。而在深地層處置場主要受到四大因素影響,包含T熱學(Thermal)、H水力(Hydraulic)、M力學(Mechanical)、C化學(Chemical)因素,稱為T-H-M-C耦合效應,通常為兩項或兩項以上交互作用,進而影響最終處置場之預期功能。
本研究針對熱-水-力耦合試驗分為小型試驗及數值模擬比對,首先小型試驗延續林柏吾(2017)小型熱-水耦合試驗並改變方式進行試驗,以先加熱後進水方式,此方式較符合於實際情況,當緩衝材料受到衰變熱影響之溫度變化進而再受到地下水入侵之模式,以時域反射法(time domain reflectometry, TDR),同時試驗不同初始乾密度(1.4 g/cm3、1.5 g/cm3、1.6 g/cm3)小型試驗,並建立視介電常數-溫度-體積含水量三相圖。但由於試驗之膨潤土具有較高的回脹壓力及回脹潛能,吸水後將產生回脹,對試體內部產生擠壓,造成孔隙改變,即乾密度的變化,可以觀察到試體底部因回脹向上擠壓,同時又將TDR感測器往上推。由於所建立之視介電常數-溫度-含水量三相圖在換算時需對應其乾密度,在乾密度改變的情況下,將會造成計算上誤差,無法反應出確實的體積含水量,因此在分層體積含水量計算上出現不符合實際情況之歷時含水量變化曲線。同時為驗證數值模擬之可信度,本研究除考慮回脹應變設定外,包含因不同溫度對對內部試體進水程度的差異,透過實際乾密度量測檢定,數值模擬之結果與量測值很相近,顯示本研究提出之數值模擬有一定的可信度,未來可針對深地層處置場情況需求進行模擬,並建立大型之數值模擬,以符合處置場的實際狀況。
摘要(英) The use of nuclear power generation has become one of the major sources of electricity in the world, but the nuclear fuel waste is tricky to treat due to its radioactive characteristic that the half-life of decay is as long as hundreds of thousands of years. Additionally, the decay heat generated during the decay process will have a temperature field effect on surroundings. How to completely isolate the used nuclear fuel from the biosphere is the common goal of all advanced nuclear energy countries. At present, the treatment for used nuclear fuel is based on the concept of “Deep Geologic Disposal”, which intends to isolate migration of radioactive species in deep formations. However, it is mainly affected by Thermal, Hydro, Mechanical, and Chemical factors, called T-H-M-C coupling effect, and usually two or more factors interact, leading the unexpected function of the final disposal site.
To access the THM coupling effects, this study proposed a small-scale physical modeling and the related numerical simulation. Firstly, the small-scale test continues Lin (2017) T-H coupling test, and the test scenario was applied in terms of heating specimen first and water intrusion subsequently. This is much in accordance with the actual situation when the buffer material is subjected to the temperature change caused by the decay heat initially and then subjected to the groundwater intrusion in field. Time domain reflectometry (TDR) was used as the core method to observe the water intrusion, and different initial dry density sets (1.4 g/cm3, 1.5 g/cm3, 1.6 g/cm3) were applied in the small-scale test. Three-dimensional diagrams of apparent dielectric constant, temperature, and volumetric water content were established accordingly. Due to the high swelling pressure of the tested bentonite, it produced re-expansion after water absorption. The inside of the specimen was squeezed, causing the changes of pores and making the dry density be changed consequently. Furthermore, it was observed that the bottom of the specimen was squeezed upward because the fixed boundary, while the TDR sensor was pushed up. Since the volumetric water content of the three-dimensional diagrams needs to correspond to dry density, calculation error produced in the case of a change in dry density. Therefore, the current observations of water content variation did not meet the actual situation.
To verify the feasibility of the numerical simulation, this study adopt influence factors of dry density changes, swelling due to saturation, and the infiltration rate as function of temperature of the internal sample. The calculations of each dry density sample were performed and similar to those of the manual sampling, indicating a certain degree of confidence in the numerical simulation. Possible future demand for the case of deep geologic disposal field simulation, and the establishment of large-scale numerical simulation to be satisfied the actual situation of the disposal field
關鍵字(中) ★ 深地質處置
★ 緩衝材料
★ 熱-水-力耦合效應
★ TDR時域反射法
★ 數值模擬
關鍵字(英) ★ Deep geological disposal
★ buffer materials
★ T-H-M coupling effects
★ time domain reflectometry
★ numerical simulation
論文目次 摘要i
目錄vi
圖目錄x
表目錄xix
第一章 緒論p.1
1.1研究動機p.1
1.2研究目的及方法p.2
第二章 文獻回顧p.5
2.1用過核子燃料深地層處置概念p.5
2.2用過核子燃料緩衝材料性質p.7
2.2.1緩衝材料概念與功能p.7
2.2.2 緩衝材料劣化性質p.10
2.3時域反射技術p.12
2.3.1物質電化學特性p.12
2.3.2 TDR量測系統與分析p.15
2.3.3 土壤電學性質與含水特性關係p.17
2.3.4 土壤電學性質與溫度關係p.19
2.4 T-H-M 耦合效應相關試驗p.20
2.4.1 西班牙相關試驗p.20
2.4.2 芬蘭相關試驗p.27
2.4.3 韓國模擬試驗p.34
2.4.4中國模擬試驗p.38
2.4.5 瑞典模擬試驗p.49
2.4.6各國T-H-M耦合試驗評析p.61
第三章-試驗材料與方法p.63
3.1試驗材料p.63
3.2儀器設備及實驗設計p.64
3.2.1 試驗相關儀器p.64
3.2.2 T-H熱水耦合模具及試驗設計p.67
3.2.3 TDR感測器製作與絕緣改良p.72
3.3.4 TDR感測器率定p.76
3.2 緩衝材料電學性質量測p.78
3.2.1膨潤土含水量控制p.78
3.2.2 視介電常數-含水量-溫度三相圖p.79
3.3 T-H小型熱水耦合試驗p.81
第四章-模擬理論及參數設定p.83
4.1程式基礎p.83
4.2 水力分析理論p.84
4.2.1 有效應力理論p.85
4.2.2 質量守恆理論p.86
4.2.3 組成行為p.88
4.2.4 滲透係數p.90
4.2.5 土壤-水份特性曲線p.92
4.2.6 水分回脹p.94
4.3 模型及參數設定p.95
4.3.1 元素網格及邊界設定p.95
4.3.2 參數設定p.98
第五章 實驗結果p.104
5.1 SPV膨潤土介電常數-溫度-含水量關係p.104
5.1.1視介電常數-溫度-含水量三相圖建立p.105
5.2 T-H小型耦合試驗結果p.109
5.2.1 初始乾密度1.4 g/cm3小型耦合試驗p.110
5.2.2 初始乾密度1.5 g/cm3小型耦合試驗p.120
5.2.3 初始乾密度1.6 g/cm3小型耦合試驗p.129
5.2.4 T-H小型耦合試驗小結p.138
5.3數值模擬分析結果p.139
5.3.1含水量模擬結果p.139
5.3.2 孔隙比模擬結果p.146
5.3.3 位移模擬結果p.150
5.4 實驗與模擬相互驗證結果p.154
第六章、結論與建議p.162
6.1結論 p.162
6.2建議 p.165
參考文獻 p.167
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指導教授 黃偉慶 鐘志忠 審核日期 2019-1-23
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