Apparent glassy dynamics of an adsorbed polymer chain in the bond-fluctuation model

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題名:	Apparent glassy dynamics of an adsorbed polymer chain in the bond-fluctuation model
作者:	Lai,PY
貢獻者:	物理研究所
關鍵詞:	LATTICE MONTE-CARLO;CRITICAL EXPONENTS;SOLID INTERFACES;FIELD-THEORY;ADSORPTION;MELTS;DIMENSIONS;SURFACE;CONFORMATIONS;SIMULATIONS
日期:	1996
上傳時間:	2010-07-08 14:07:10 (UTC+8)
出版者:	中央大學
摘要:	The dynamics of a single homopolymer chain strongly adsorbed on a flat surface is investigated by Monte Carlo simulation using the bond-fluctuation model. Previously observed anomalous glassy dynamics at low temperatures [Phys. Rev. E 49, 5420 (1994)] is revisited in detail. We also study the dynamics of a polymer chain confined in a narrow slit of width of a monomer and a modified bond-fluctuation model in three dimensions to include more relevant bond vectors. We show that the previously observed glassy dynamics is due to an artifact of the bond-fluctuation model in three dimensions in that it does not cross-over to the two dimensional bond-fluctuation model with the correct Rouse dynamics. With the proper inclusion of the extra bond vectors P(2,2,0) and P(3,2,0), no glassy behavior appears for the strongly adsorbed chain.
關聯:	MACROMOLECULAR THEORY AND SIMULATIONS
顯示於類別:	[物理研究所] 期刊論文

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