博碩士論文 102226045 詳細資訊




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姓名 簡仲信(Chien chung-hsin)  查詢紙本館藏   畢業系所 光電科學與工程學系
論文名稱 基於鈉鉀離子交換波導之光學力推動金奈米球
(Optical Propulsion of Gold Nanoparticles Based on Na+-K+ Ion Exchanged Waveguide)
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摘要(中) 本論文利用鈉鉀離子交換的技術製作光波導當作光推球基板,並藉由顯微鏡系統研究金奈米粒子受到波導表面消逝場時的運動情形。在理論上模擬金奈米球在波導消逝場上的受力行為,並指出奈米系統下的化學效應對於穩定地捕陷以及推動奈米粒子的重要性。在實驗上我們成功地捕陷並推動二氧化矽微米球超過140微米的距離,然而對於金奈米球而言,雖然其推動和布朗運動相比是明顯的,但是穩定地捕陷以及推動是不成功的。我們將其歸因於波導上方消逝場的侷限性不足,未來使用表面電漿型式的光波導可以大大地改善缺失。
摘要(英) In this study, the propulsion of colloidal gold nanoparticles based on Na+-K+ ion exchange waveguides via the evanescent field was analyzed. Theoretically, the approach to calculate the optical forces exerted on nanoparticles was reviewed. Of particularly interest, we point out the importance where the chemistry of the nanoscale environment should be specially tailored in order to achieve trapping and transport of nanoparticles with high stability. Experimentally, we demonstrate the propulsion of silica micrometer-sized spheres along the optical waveguide over a length of 140μm. On the contrary, although the movement of gold nanoparticles against brownian motion was obvious, stable trapping and transport was not successful. We attribute the result to relatively weak gradient forces which can be further improved utilizing surface plasmon polariton waveguides.
關鍵字(中) ★ 光操控
★ 光推動
★ DLVO理論
★ 布朗運動
★ 消逝場
★ 金奈米粒子
關鍵字(英) ★ Optical manipulation
★ Optical propulsion
★ DLVO theory
★ Brownian motion
★ evanescent field
★ gold nanoparticles
論文目次 中文摘要 I
Abstract II
誌謝 III
目錄 i
圖目錄 iv
表目錄 viii
第一章 緒論 1
1-1 前言 1
1-2 歷史背景 4
1-3 文獻回顧 4
1-4 研究動機 9
1-5 論文架構 11
第二章 研究方法 12
2-1 羅倫茲-杜德模型 12
2-2 米氏理論 18
2-2-1米氏理論簡介 18
2-2-2米氏理論推導 19
2-2-3平面波激發 25
2-2-4消逝波激發 29
2-2-5瑞利理論近似 31
2-2-6極化率表示式 32
2-2-7模擬結果與討論 35
2-3 光學力 38
2-3-1光學力簡介 38
2-3-2羅倫茲力推導 39
2-3-3消逝場的形式 40
2-3-4模擬結果 41
2-4 非光學力 45
2-4-1非光學力簡介 45
2-4-2史托克斯定律 45
2-4-3重力與浮力 48
2-4-4布朗運動 49
2-4-5 DLVO理論 51
2-5波導理論 62
2-5-1波導簡介 62
2-5-2離子交換法 64
2-5-3光束傳播法 71
第三章 實驗設計與架構 72
3-1 波導製作 72
3-2 實驗架構 76
3-3 實驗參數 80
3-4 實驗模擬 87
第四章 實驗結果與討論 91
4-1 實驗原型 91
4-2 改變黏滯係數 100
4-3 二氧化矽微米球 102
第五章 結論與未來展望 104
5-1 結論 104
5-2 未來與展望 105
參考文獻 106
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指導教授 戴朝義(Tai Chao-yi) 審核日期 2016-7-15
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