垃圾焚化爐空氣污染控制設備影響戴奧辛排放特性之初步探討

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林忠正(Jung-Jeng Lin) 查詢紙本館藏

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論文名稱

垃圾焚化爐空氣污染控制設備影響戴奧辛排放特性之初步探討
(The Effects of Air Pollution Control Devices on the Dioxin Emissions from Municipal Waste Incinerators)

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關鍵字(中)

★ 戴奧辛
★ 都市垃圾焚化爐
★ 活性碳

關鍵字(英)

★ Dioxins
★ PCDDs
★ PCDFs
★ Municipal Waste Incinerator
★ Activated Carbon

論文目次

摘要 I
ABSTRACT II
目錄 III
圖目錄 VII
表目錄 X
相關名詞及單位符號 XIII
第一章前言 1
1.1研究緣起 1
1.2研究目的與範疇 2
第二章文獻回顧 3
2.1 戴奧辛的基本性質與特徵 3
2.2焚化爐中戴奧辛的生成機制 6
2.2.1 前驅物異相催化反應 7
2.2.2 de novo合成反應 9
2.3 國內外焚化廠戴奧辛排放之管制規範 11
2.3.1 大氣中戴奧辛來源 11
2.3.2 世界各國對焚化廠排放戴奧辛之管制措施 12
2.3.3 焚化廠戴奧辛排放控制技術 24
2.4 國內外焚化廠APCD與戴奧辛排放量 43
2.4.1 國外焚化廠APCD與戴奧辛排放量的比較 43
2.4.2 國內焚化廠與戴奧辛排放量的比較 44
第三章研究方法 52
3.1 研究流程設計 52
3.2 實驗藥品與試劑 52
3.2.1 實驗藥品 52
3.2.2 實驗溶劑 54
3.3 實驗材料與設備 55
3.3.1 實驗材料 55
3.3.2 實驗設備 56
3.4 採樣方法 56
3.4.1 樣品瓶之清洗程序 57
3.4.2 煙道採樣流程 58
3.4.3 灰樣品採樣程序 72
3.5 戴奧辛分析方法 72
3.5.1 樣品前處理 72
3.5.2 分析儀器條件之設定 76
3.6 氯鹽分析方法 84
第四章結果與討論 86
4.1 HRGC/LRMS分析戴奧辛 86
4.1.1 滯留時間窗建立 86
4.1.2 建立檢量線與啟始校正 87
4.1.3 氣象層析管柱解析度測試 87
4.1.4 儀器靈敏度測試（雜訊比規範） 88
4.1.5 檢量線離子強度比與相對感應因子計算 88
4.1.6 滯留時間規範 89
4.2 兩廠戴奧辛排放濃度比較 102
4.2.1 空氣污染防制設備前之戴奧辛濃度 102
4.2.2 煙囪排放之戴奧辛濃度 111
4.3 兩廠戴奧辛排放量比較 116
4.3.1 APCD前後戴奧辛濃度及毒性當量濃度的變化 116
4.3.2 APCD對戴奧辛濃度及毒性當量濃度的去除效率 117
4.4 記憶效應對B廠戴奧辛排放濃度之影響 121
4.4.1 B廠間隔一年之APCD前戴奧辛排放濃度比較 121
4.4.2 B廠間隔一年之煙囪戴奧辛排放濃度比較 125
4.5 戴奧辛各物種貢獻度之變化 134
4.6 與國外焚化源排放戴奧辛物種比較 135
4.7 分階粒徑微粒上氯鹽含量與戴奧辛的關係 144
4.8 飛灰中戴奧辛濃度 145
4.8.1 集塵器飛灰中戴奧辛比較 145
4.8.2 焚化爐排出之戴奧辛分佈比例計算 146
第五章結論與建議 151
5.1結論 151
5.2 建議 152
參考文獻 154
附錄A 品保查核項目圖譜
附錄B 樣品回收率品質管制圖

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指導教授

張木彬(Moo-Been Chang)

審核日期

2000-7-13

推文