電漿驅動器臭氧生成之研究

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童保舜(Bao-shun Tong) 查詢紙本館藏

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論文名稱

電漿驅動器臭氧生成之研究
(Investigation on Ozone Formation with Plasma Actuator)

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摘要(中)

過去有關電漿驅動器之研究多著重於電極表面之空氣動力特性，尚未針對電漿驅動器於運作時產生之臭氧濃度做探討，本研究利用電漿驅動器在不同參數下產生之臭氧濃度做深入之了解，討論操作參數改變對於臭氧濃度所造成之影響。並以數值模式模擬不同之操作參數產生之臭氧濃度，找出電漿驅動器中控制臭氧濃度之重要因子，以期充分掌握電漿驅動器之臭氧生成特性。
　　由本研究結果得知，以純氧為工作氣體時臭氧濃度會是以空氣為工作氣體時之2.5倍；而放電功率、施加電壓與供電頻率之上升皆會使臭氧濃度上升；驅動器之幾何外形（如：電極構造、電極長度）亦會造成臭氧濃度明顯之改變；折合電場在約160 Td時臭氧濃度為最高值，不管折合電場增加或減少臭氧濃度皆會下降；溫度效應則是當溫度越高時，臭氧濃度會越低。
　　由最適化條件來看，在兼顧電漿驅動器效能與臭氧濃度之參數為介電質為KaptonR，頻率為1 kHz，施加電壓為16 kV，電極長度為80 mm，電極構造為6-3-6，所生成之臭氧濃度為119 ppm。
　　能源效率之計算結果顯示當頻率上升時，能源效率會有下降之趨勢，而又以施加電壓為19kV時下降趨勢最為明顯，且電漿驅動器之能源效率在同型反應器中為最小值，亦即在實際應用時會生成最少之臭氧，可降低對環境之危害。

摘要(英)

In recent years, several studies have focused on the actuator changed the effect of aerodynamic characteristics, but without any research focused on ozone formation that plasma actuator generated. This study is focused on the characteristics of ozone formation with DBD plasma actuator and investigated with experimental tests and numerical model. Experimental results indicate that discharge power, frequency, electrode configuration, dielectric and applied voltage would affect ozone formation significantly. Numerical results show that discharge power, reduced field and temperature are factors affecting ozone formation with plasma actuator. In this study also conduct the energy efficiency of plasma actuator, it shows that plasma actuator has the minimum energy efficiency compared with the same type reactors.

關鍵字(中)

★ 能源效率
★ 最適化條件
★ 數值模式
★ 臭氧
★ 電漿驅動器

關鍵字(英)

★ ozone formation
★ numerical model
★ energy efficiency
★ Plasma actuator

論文目次

摘要　　　　　　　　　　　　　　　　　　　　i
Abstract 　　　　　　　　　　ii
誌謝　　　　　　　　　　　　　　　iii
目錄　　　　　　　　　　　　　　　v
圖目錄　　　　　　　　　　　　　　　viii
表目錄　　　　　　　　　　　　　　　x
第一章　前言　　　　　　　　　　　　　　　1
　1.1　研究緣起　　　　　　　　　　　　　　　1
　1.2　研究目的　　　　　　　　　　　　　　　2
第二章文獻回顧　　　　　　　　　　　　　　　3
　2.1　電漿　　　　　　　　　　　　　　　3
　　2.1.1　電漿反應　　　　　　　　　　5
　　2.1.2　折合電場　　　　　　　　　　6
　　2.1.3　G-value 　　　　　　　　　　7
　　2.1.4　電漿應用　　　　　　　　　　8
　　2.1.5　非熱電漿種類　　　　　　　　　　8
　2.2　臭氧　　　　　　　　　　　　　　　15
　　2.2.1　臭氧基本性質　　　　　　　　　　15
　　2.2.2　臭氧的危害性　　　　　　　　　　16
　　2.2.3　臭氧在空氣中的衰減　　　　　17
　　2.2.4　臭氧在生活中應用　　　　　　　　　　17
　　2.2.5　參數影響　　　　　　　　　　18
　　2.2.6　臭氧在DBD系統中主要生成與破壞機制 21
　2.3　電漿驅動器　　　　　　　　　　　　　　　24
　　2.3.1　基本原理　　　　　　　　　　24
　　2.3.2　介電質放電電漿驅動器　　　　　25
　　2.3.3　電暈放電電漿驅動器　　　　　27
　　2.3.4　近來電漿驅動器之研究　　　　　28
　2.4　數值模式　　　　　　　　　　　　　　　29
第三章實驗方法　　　　　　　　　　　　　　　34
　3.1　實驗設備　　　　　　　　　　　　　　　34
　　3.1.1　實驗配置　　　　　　　　　　34
　　3.1.2　氣體　　　　　　　　　　　　　　　35
　　3.1.3　電漿驅動器　　　　　　　　　　35
　　3.1.4　高壓電力供應系統　　　　　　　　　　36
　　3.1.5　偵測系統　　　　　　　　　　38
　3.2　數值模式　　　　　　　　　　　　　　　40
　　3.2.1　資料輸入　　　　　　　　　　42
　　3.2.2　Boltzmann方程式求解工具　　　　　43
　　3.2.3　理論崩潰電壓與放電功率之計算 48
　　3.2.4　反應式與速率常數資料庫　　　　　49
　　3.2.5　反應途徑分析　　　　　　　　　　51
　　3.2.6　反應方程式　　　　　　　　　　52
第四章結果與討論　　　　　　　　　　53
　4.1　實驗結果　　　　　　　　　　　　　　　53
　　4.1.1　放電情形　　　　　　　　　　54
　　4.1.2　波型　　　　　　　　　　　　　　　54
　　4.1.3　工作氣體對於臭氧濃度之影響　　　　　55
　　4.1.4　頻率對於臭氧濃度之影響　　　　　57
　　4.1.5　施加電壓對於臭氧濃度之影響　　　　　59
　　4.1.6　電極幾何外形對於臭氧濃度之影響 61
　　4.1.7　放電功率對於臭氧濃度之影響　　　　　63
　　4.1.8　介電質對於臭氧濃度之影響　　　　　65
　4.2　數值模式　　　　　　　　　　　　　　　67
　　4.2.1　工作氣體對於臭氧濃度之影響　　　　　67
　　4.2.2　折合電場對於臭氧濃度之影響　　　　　68
　　4.2.3　氣體溫度對於臭氧濃度之影響　　　　　70
　4.3　最佳化條件探討　　　　　　　　　　72
　4.4　電漿驅動器之能源效率　　　　　　　　　　75
第五章結論與建議　　　　　　　　　　77
　5.1　結論　　　　　　　　　　　　　　　77
　5.2　建議　　　　　　　　　　　　　　　78
參考文獻　　　　　　　　　　　　　　　79
附錄一數值模擬中使用之反應式及速率常數 91

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指導教授

張木彬(Moo-been Chang)

審核日期

2012-8-25

推文