考慮異質性膨潤土內氣體遷移之多相流與力學耦合數值模擬

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林禹昇(Yu-Sheng Lin) 查詢紙本館藏

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應用地質研究所

論文名稱

考慮異質性膨潤土內氣體遷移之多相流與力學耦合數值模擬
(Numerical Simulation of Coupled Multiphase Fluid Flow and Mechanics for Gas Migration in Bentonite Considering Heterogeneous Distributions)

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至系統瀏覽論文 (2026-8-1以後開放)

摘要(中)

高階放射性廢棄物最終處置方式為深層地質處置，以多重障壁概念，將廢棄物包覆在處置罐中，並運至地層至少三百公尺以下的岩體中，再填滿緩衝材料，藉由隔離、遲滯原理以確保廢棄物衰變到無害程度，與生物圈隔離，保護民眾健康及環境安全。然而，經處置數百年後，廢棄物自身衰變產生熱，處置系統溫度隨之上升，熱膨脹使應力改變，進而造成水力及化學效應產生。在低氧環境下金屬廢棄物罐腐蝕、輻解作用、微生物降解均可能產生氣體，隨著氣體持續累積，一旦作用在緩衝材料上的應力無法承受氣體壓力，孔隙將逐漸擴張並產生裂隙，氣體藉此流出至岩體，影響處置系統之能力，造成安全性的危險。因此，緩衝材料在系統中扮演著極為關鍵的角色，膨潤土為常見的緩衝材料選擇，在實際情況下，膨潤土含有不同的顆粒排列、孔隙率和滲透率，呈現異質性的空間分佈，這種異質性可能在高孔隙率及疏鬆顆粒排列之區域，形成優先通道，使氣體更容易流通，進而影響氣體的遷移行為。因此，本研究成功地利用THMC7.1數值模式顯示氣體壓力累積之變化，並以異質性膨潤土進行模擬，其結果確定異質性分佈所產生的氣體優先通道確實會影響氣體速度。

摘要(英)

The final disposal method for high-level waste is Deep Geological Disposal. This is where nuclear waste is buried in geological formations at depths greater than 300 meters, and canister and buffer materials are used to cover and secure it. By the principles of isolation and retardation, the waste decays harmlessly, isolating it from the biosphere and ensuring human health and environmental safety. However, after hundreds of years of disposal, gas may be generated due to the corrosion of metallic materials under anoxic conditions, the radiolysis of water or microbial degradation. With continuous gas pressure accumulation, the stress on buffer materials can no longer withstand it, leading to pathway dilation and fractures, allowing gas to escape. As gas degrades the barrier′s capability, endangering the safety of the repository. Therefore, buffer materials play a crucial role in the repository, bentonite is commonly chosen as the buffer materials. In practical situations, bentonite exhibits different particle arrangements, porosity, and permeability, presenting heterogeneous distributions. This heterogeneity may lead to the formation of preferential pathways, particularly in regions with high porosity and loose particle arrangements, making gas flow more accessible and consequently influencing the gas migration behavior. Therefore, this study successfully utilized the THMC7.1 numerical model to demonstrate the changes in gas pressure accumulation. Simulations with heterogeneous bentonite confirmed that the preferential pathways created by heterogeneous distribution significantly affect gas velocity.

關鍵字(中)

★ 深層地質處置
★ 異質性膨潤土
★ 氣體遷移
★ 多相流
★ 耦合數值模擬

關鍵字(英)

★ Deep Geological Disposal
★ Heterogeneous bentonite
★ Gas migration
★ Multiphase fluid flow
★ Coupled numerical simulation

論文目次

摘要 i
ABSTRACT ii
致謝 iii
圖目錄 vii
表目錄 x
符號說明 xi
一、緒論 1
1-1前言 1
1-2研究目的 2
1-3研究流程 2
二、文獻回顧 4
2-1高放射性廢棄物處置概念 4
2-2熱-水-力-化耦合關係 6
2-3氣體形成與遷移之影響 9
三、分析理論與數值模擬方法 14
3-1多相流體相關理論 14
3-1-1飽和度 15
3-1-2利用界面張力和接觸角判斷流體之濕潤度 15
3-1-3毛細壓力與飽和度之間關係 16
3-1-4 Darcy定律 22
3-1-5經驗公式 26
3-2 THMC7.1數值模式介紹 30
3-3 THMC7.1數值模式之控制方程式 31
3-3-1多相流模組 31
3-3-2熱傳模組 36
3-3-3力學模組 37
3-3-4化學模組 39
3-4耦合熱傳-多相流-力學-化學分析 40
四、結果與討論 41
4-1實驗室實驗數據 41
4-2模型建置 45
4-3網格收斂性分析 46
4-4參數敏感度分析 49
4-5模擬設定 53
4-5-1網格設定 53
4-5-2參數設定 54
4-5-3初始條件 57
4-5-4邊界條件 58
4-6模擬結果與討論 62
4-6-1參數率定 62
4-6-2模擬結果 64
4-7考慮異質性膨潤土之結果與討論 70
4-7-1利用滲透率設定之結果 71
4-7-2利用孔隙率設定之結果 73
五、結論與建議 75
5-1結論 75
5-2建議 76
參考文獻 77
附錄A 80
附錄B 83
B-1 THMC7.1數值模式演進歷程 83
B-2有限元素法 84
B-2-1基本概念 84
B-2-2元素形狀 84
B-2-3加權殘餘法 87
B-2-4 Galerkin法 90
B-2-5有限元素法之控制方程式推導 90

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指導教授

陳瑞昇(Jui-Sheng Chen)

審核日期

2024-7-15

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