Random styrenic copolymers with pendant pyrene moieties: Synthesis and applications in organic field-effect transistor memory

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Title:	Random styrenic copolymers with pendant pyrene moieties: Synthesis and applications in organic field-effect transistor memory
Authors:	劉振良;Chung, Fei-Jan;Liu, Hsin-Yu;Jiang, Bo-Yi;He, Guan-Yu;Wang, Shi-Hao;Wu, Wen-Chung;Liu, Cheng-Liang
Contributors:	工學院化學工程與材料工程學系
Keywords:	composite polymers;computer hardware;Copolymers;Data storage;donor;electret;Electrets;electrical properties;electrochemistry;Field effect transistors;Jewelry;memory;pendant copolymers;Semiconductor devices;styrene;Styrenes;transistor;Trapping
Date:	2016-04-01
Issue Date:	2026-04-21 14:50:44 (UTC+8)
Publisher:	John Wiley and Sons Inc.;Hoboken: Wiley
Abstract:	摘要： Three random copolymers comprised pendant styrene and 4‐(1‐pyrenyl)‐styrene (PyS) moieties in different molar ratios (21.4:1 (P1), 3.9:1 (P2), and 1.4:1 (P3)) were synthesized and employed as charge storage polymeric electret for nonvolatile organic field‐effect transistor (OFET) memory application. The impact of varying the molar ratio in side‐chain electron‐donating pyrene moieties on the thermal, optical, photophysical, electrochemical, and electrical properties of the resulting pendant copolymers was evaluated to establish structure–property relationship. The OFET memory with P3 electret layer exhibits a largest memory window of 41.8 V, long retention time of 10⁴ s with memory ratio of 10⁵, and stable reversibility of at least 100 cycles due to enhanced field‐induced holes trapping ability from higher PyS composition ratio. Therefore, polymer electret with pendant functional moieties shows potential for use as trapping layer in OFET memory devices. © 2015 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2016, 54, 910–917 其他題名： J. Polym. Sci. Part A: Polym. Chem 出版者： Hoboken: Wiley 出版日期： 2016-04-01 出處： Journal of polymer science. Part A, Polymer chemistry, 2016-04, Vol.54 (7), p.910-917 版權： 2015 Wiley Periodicals, Inc. 版權： 2016 Wiley Periodicals, Inc. 識別號： ISSN: 0887-624X 識別號： EISSN: 1099-0518 識別號： DOI: 10.1002/pola.27995 識別號： CODEN: JPACEC
Appears in Collections:	[Department of Chemical and Materials Engineering] journal & Dissertation

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